In optics, various autocorrelation functions can be experimentally realized. The field autocorrelation may be used to calculate the spectrum of a source of light, while the intensity autocorrelation and the interferometric autocorrelation are commonly used to estimate the duration of ultrashort pulses produced by modelocked lasers. The laser pulse duration cannot be easily measured by optoelectronic methods, since the response time of photodiodes and oscilloscopes are at best of the order of 200 femtoseconds, yet laser pulses can be made as short as a few femtoseconds.
In the following examples, the autocorrelation signal is generated by the nonlinear process of second-harmonic generation (SHG). Other techniques based on two-photon absorption may also be used in autocorrelation measurements, as well as higher-order nonlinear optical processes such as third-harmonic generation, in which case the mathematical expressions of the signal will be slightly modified, but the basic interpretation of an autocorrelation trace remains the same. A detailed discussion on interferometric autocorrelation is given in several well-known textbooks.
