Fission products in the context of "Fallout"

Nuclear fallout is residual radioisotope material that is created by the reactions producing a nuclear explosion or nuclear accident. In explosions, it is initially present in the radioactive cloud created by the explosion, and "falls out" of the cloud as it is moved by the atmosphere in the minutes, hours, and days after the explosion. The amount of fallout and its distribution is dependent on several factors, including the overall yield of the weapon, the fission yield of the weapon, the height of burst of the weapon, and meteorological conditions.

Fission weapons and many thermonuclear weapons use a large mass of fissionable fuel (such as uranium or plutonium), so their fallout is primarily fission products, and some unfissioned fuel. Cleaner thermonuclear weapons primarily produce fallout via neutron activation. Salted bombs, not widely developed, are tailored to produce and disperse specific radioisotopes selected for their half-life and radiation type.

In nuclear astrophysics, the rapid neutron-capture process, also known as the r-process, is a set of nuclear reactions that is responsible for the creation of approximately half of the atomic nuclei heavier than iron, the "heavy elements", with the other half produced largely by the s-process. The r-process synthesizes the more neutron-rich of the stable isotopes of even elements, and those separated from the beta-stable isotopes by those that are not often have very low s-process yields and are considered r-only nuclei; the heaviest isotopes of most even elements from zinc to mercury fall into this category. Abundance peaks for the r-process occur near mass numbers A = 82 (elements Se, Br, and Kr), A = 130 (elements Te, I, and Xe) and A = 196 (elements Os, Ir, and Pt). Further, all the elements heavier than bismuth, including natural thorium and uranium (and other actinides) must ultimately originate in an r-process nucleus.

The r-process entails a succession of rapid neutron captures (hence the name) by one or more heavy seed nuclei, typically beginning with nuclei in the abundance peak centered on Fe. The captures must be rapid in the sense that the nuclei must not have time to undergo radioactive decay (typically via β decay) before another neutron arrives to be captured. This sequence can continue up to the limit of stability of the increasingly neutron-rich nuclei (the neutron drip line) to physically retain neutrons as governed by the short range nuclear force. The r-process therefore must occur in locations where there exists a high density of free neutrons. At some time following the neutron captures, the nucleus beta-decays back to the line of stability (just as with fission products) resulting in a stable isotope of the same mass number A, and normally the most neutron-rich of those.

High-level waste (HLW) is a type of nuclear waste created by the irradiation of nuclear fuel in a reactor. Irradiation causes a build-up of fission products and transuranic elements (generated by capture of neutrons) in the fuel. Fission products typically have a much shorter half-life than uranium, which means the irradiated fuel is more radioactive and thus hotter than fresh fuel – high-level waste has heat output of >2 kW/m. At the same time, the fissile material (usually uranium-235) is used up, so that the fuel is no longer able to sustain the operation of the reactor and must be recycled or disposed of as waste.

High-level waste includes spent nuclear fuel itself as well as the byproducts of nuclear reprocessing, which results in liquid raffinates and other waste streams. Liquid wastes are not suitable for disposal, so these are vitrified to convert them into a solid, glass form which is suitable for disposal.

Nuclear reprocessing is the chemical separation of fission products and actinides from spent nuclear fuel. Originally, reprocessing was used solely to extract plutonium for producing nuclear weapons. With commercialization of nuclear power, the reprocessed plutonium was recycled back into MOX nuclear fuel for thermal reactors. The reprocessed uranium, also known as the spent fuel material, can in principle also be re-used as fuel, but that is only economical when uranium supply is low and prices are high. Nuclear reprocessing may extend beyond fuel and include the reprocessing of other nuclear reactor material, such as Zircaloy cladding.

The high radioactivity of spent nuclear material means that reprocessing must be highly controlled and carefully executed in advanced facilities by specialized personnel. Numerous processes exist, with the chemical based PUREX process dominating. Alternatives include heating to drive off volatile elements, burning via oxidation, and fluoride volatility (which uses extremely reactive Fluorine). Each process results in some form of refined nuclear product, with radioactive waste as a byproduct. Because this could allow for weapons grade nuclear material, nuclear reprocessing is a concern for nuclear proliferation and is thus tightly regulated.

Radiological warfare is any form of warfare involving deliberate radiation poisoning or contamination of an area with radioisotopes, but without the use of nuclear weapons. While radiological weapons were researched and in some cases tested during the Cold War, there is no evidence any military has ever deployed operational radiological weapons, although they have been used for assassination.

Nuclear warfare, both via fission and fusion weapons, creates radioisotopes in the form of fission products and neutron-activated surface material. This fallout is incorporated into military planning. Neutron bombs are designed to maximize the lethal radiation area and minimize the blast. These uses are generally not considered direct radiological warfare, but salted bombs, which maximize radioisotope production in a nuclear blast, are.